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EdgeFiller
Selective edge filling of collapsed carbon nanotubes for nanoelectronics
FunderFrench National Research Agency (ANR)
Funder Contribution €521,100.00
DurationFrom 01 Oct 2016
Project codeANR-16-CE24-0008
Identifiers
Description
EdgeFiller proposes an innovative way to create collapsed carbon nanotubes for use as a highly adaptable superior alternative to conventional graphene nanoribbons, currently proposed as a key component for future electronics. These new nanoribbons will be prepared by extracting the outer wall from large multi-walled carbon nanotubes via techniques patented by project partners. These large single-walled nanotubes (SWCNT) spontaneously collapse due to their diameter and are referred to as “dogbones” due to the cross-sectional shape they adopt, with nanometric tubular cavities at each side surrounding a central flat region. The properties of these new hybrid materials, between graphene and SWCNTs, comes from these cavities along the edges, which will be filled with material such as salts (KI, …), molecules (C60, TCNQ, TTF, …), or metals. This allows doping (charge and/or spin) of the ribbon without introducing defects or scattering centres, a critical “roadblock” to current utilization of both graphene and SWCNTs taken separately. This will result in a wide range of different electrical and optoelectronic behaviour. In the project, we aim to control both the conductivity this way, the p- ou n- character of charge carriers, and introduce high-mobility spin carriers. The edge cavity filling can either be symmetry, or asymmetric (one side acceptor, the other donor), based on an innovative method we propose to develop, to create nanoribbons with strong transversal electric fields. The technique promises a cheap and easily upscalable approach resolving many of the current blockages to graphene- and nanotube-based devices. EdgeFiller brings together three world leading CNRS nanocarbon groups to develop this innovative concept, covering all fields from theoretical DFT modelling, through filled ribbon production, to a demonstration device (a prototype FET).
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EdgeFiller proposes an innovative way to create collapsed carbon nanotubes for use as a highly adaptable superior alternative to conventional graphene nanoribbons, currently proposed as a key component for future electronics. These new nanoribbons will be prepared by extracting the outer wall from large multi-walled carbon nanotubes via techniques patented by project partners. These large single-walled nanotubes (SWCNT) spontaneously collapse due to their diameter and are referred to as “dogbones” due to the cross-sectional shape they adopt, with nanometric tubular cavities at each side surrounding a central flat region. The properties of these new hybrid materials, between graphene and SWCNTs, comes from these cavities along the edges, which will be filled with material such as salts (KI, …), molecules (C60, TCNQ, TTF, …), or metals. This allows doping (charge and/or spin) of the ribbon without introducing defects or scattering centres, a critical “roadblock” to current utilization of both graphene and SWCNTs taken separately. This will result in a wide range of different electrical and optoelectronic behaviour. In the project, we aim to control both the conductivity this way, the p- ou n- character of charge carriers, and introduce high-mobility spin carriers. The edge cavity filling can either be symmetry, or asymmetric (one side acceptor, the other donor), based on an innovative method we propose to develop, to create nanoribbons with strong transversal electric fields. The technique promises a cheap and easily upscalable approach resolving many of the current blockages to graphene- and nanotube-based devices. EdgeFiller brings together three world leading CNRS nanocarbon groups to develop this innovative concept, covering all fields from theoretical DFT modelling, through filled ribbon production, to a demonstration device (a prototype FET).
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