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CollZSiC
Design of core/shell: ZrC/SiC nanocomposites
FunderFrench National Research Agency (ANR)
Funder Contribution €594,775.00
DurationFrom 01 Feb 2013
Project codeANR-12-BS08-0004
Identifiers
Description
The present project deals with the development of new core-shell ZrC/SiC nanocomposites. The elaboration of these non-oxide systems with an original structure is a real challenge considering the synthetic approaches, and could present a strong point of interest in the use of structural materials, in the nuclear and the aeronautic domains or the steel industry. These systems will be synthesized from original polycarbosilanes (PCSs), precursors of SiC ceramics, coating mineral particles of zirconium carbide obtained by carboreduction of zirconia. The new generation of core-shell nanoparticles will be realised thanks to the laser-pyrolysis method. During each step of the process of synthesis, a theoretical approach of the surface phenomena will be undertaken using the density functional theory (DFT) combined with fine structural analysis. This pluridisciplinary project combines several complementary research laboratories with skills recognised nationality and internationality. The SPCTS laboratory at the University of Limoges has expertise in the synthesis and characterization of composites made from organic-inorganic hybrid systems. The UCCS at the University of Lille has specific skills in the DFT study and the characterisation of inorganic surfaces. The LCMCP at the University Pierre et Marie Curie (Paris 6) has extensive experience in the characterisation of pre-ceramic polymer and surface covalent bonds. Finally, the Francis Perrin laboratory has significant know-how in the generation of non-oxide nano-objects using the laser pyrolysis technique. On a scientific level and in addition to obtaining original nanoparticle systems of interest, the objectives are the control of: - the functionalization of ZrC surfaces; - the grafting of organic macromolecules onto the surface of mineral particles; - the development of hybrid suspensions suitable for pyrolysis-laser; - the systematic understanding through modelling, of properties and mechanisms at surfaces and interfaces. On the one hand, this project should help to improve knowledge in the field of non-oxide core-shell nanostructures, using an approach combining characterization and modelling. On the other hand, it should open new perspectives for applications in the above areas namely the nuclear, the aeronautic and the steel industry.
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The present project deals with the development of new core-shell ZrC/SiC nanocomposites. The elaboration of these non-oxide systems with an original structure is a real challenge considering the synthetic approaches, and could present a strong point of interest in the use of structural materials, in the nuclear and the aeronautic domains or the steel industry. These systems will be synthesized from original polycarbosilanes (PCSs), precursors of SiC ceramics, coating mineral particles of zirconium carbide obtained by carboreduction of zirconia. The new generation of core-shell nanoparticles will be realised thanks to the laser-pyrolysis method. During each step of the process of synthesis, a theoretical approach of the surface phenomena will be undertaken using the density functional theory (DFT) combined with fine structural analysis. This pluridisciplinary project combines several complementary research laboratories with skills recognised nationality and internationality. The SPCTS laboratory at the University of Limoges has expertise in the synthesis and characterization of composites made from organic-inorganic hybrid systems. The UCCS at the University of Lille has specific skills in the DFT study and the characterisation of inorganic surfaces. The LCMCP at the University Pierre et Marie Curie (Paris 6) has extensive experience in the characterisation of pre-ceramic polymer and surface covalent bonds. Finally, the Francis Perrin laboratory has significant know-how in the generation of non-oxide nano-objects using the laser pyrolysis technique. On a scientific level and in addition to obtaining original nanoparticle systems of interest, the objectives are the control of: - the functionalization of ZrC surfaces; - the grafting of organic macromolecules onto the surface of mineral particles; - the development of hybrid suspensions suitable for pyrolysis-laser; - the systematic understanding through modelling, of properties and mechanisms at surfaces and interfaces. On the one hand, this project should help to improve knowledge in the field of non-oxide core-shell nanostructures, using an approach combining characterization and modelling. On the other hand, it should open new perspectives for applications in the above areas namely the nuclear, the aeronautic and the steel industry.
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Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. 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Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. 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Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. 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