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AMSTOR
Aminated 2D BN nanosheets for H2 storage
FunderFrench National Research Agency (ANR)
Funder Contribution €518,810.00
DurationFrom 01 Apr 2025
Project codeANR-24-CE09-6152
Identifiers
Description
The AMSTOR project is dedicated to the development of aminated 2D boron nitride nanosheets in view of hydrogen solid-state storage by physisorption, with high gravimetric capacity (>10wt%) and moderate desorption temperatures (<150°C). This project will be spread over a period of 36 months and will involve 2 laboratories (Laboratoire de Nanomédeince EA 4662 de l’université de Besançon et Institut européen des membranes de L’université de Montpellier) and a company involved in H2 storage (Mahytec, France). It is part of the “management of nano-scale interfaces, functionalization and interaction between nano-scale interfaces”. Hexagonal boron nitride (h-BN) nanosheets can be aminated by alkylamide salts (Li or Na) via a one pot process in mild conditions, limiting the cost of the process. The aminated h-BN nanosheets by alkylamide are promising candidates for H2 uptake thanks to ion doping and amine functionalization while keeping their chemical stability. Therefore, our chemical process to functionalize h-BN nanosheets brings a new approach to search an optimal hydrogen uptake. This has not yet been reported. Our goal is thus to find the optimal combinations of gravimetric and volumetric uptakes versus geometry, temperature, pressure, grafting and doping. As such, our aminated h-BN nanosheets must address the inherent challenges of functionalized ultra-thin 2D materials for H2 uptake to meet the DoE criteria. Despite a wide range of solid-state materials, including 2D materials, there is still a need for high performance H2 storage. To address this issue, volumetric experimental set-up will be used for industrial test benches and characterize hydrogen storage. Ab initio calculations coupled to molecular dynamics (AIMD) will support experimental measurements from modelization of the adsorption sites to explain isotherm experiments. Then, a technical-economic study will be conducted to position aminated h-BN nanosheets for H2 storage.
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The AMSTOR project is dedicated to the development of aminated 2D boron nitride nanosheets in view of hydrogen solid-state storage by physisorption, with high gravimetric capacity (>10wt%) and moderate desorption temperatures (<150°C). This project will be spread over a period of 36 months and will involve 2 laboratories (Laboratoire de Nanomédeince EA 4662 de l’université de Besançon et Institut européen des membranes de L’université de Montpellier) and a company involved in H2 storage (Mahytec, France). It is part of the “management of nano-scale interfaces, functionalization and interaction between nano-scale interfaces”. Hexagonal boron nitride (h-BN) nanosheets can be aminated by alkylamide salts (Li or Na) via a one pot process in mild conditions, limiting the cost of the process. The aminated h-BN nanosheets by alkylamide are promising candidates for H2 uptake thanks to ion doping and amine functionalization while keeping their chemical stability. Therefore, our chemical process to functionalize h-BN nanosheets brings a new approach to search an optimal hydrogen uptake. This has not yet been reported. Our goal is thus to find the optimal combinations of gravimetric and volumetric uptakes versus geometry, temperature, pressure, grafting and doping. As such, our aminated h-BN nanosheets must address the inherent challenges of functionalized ultra-thin 2D materials for H2 uptake to meet the DoE criteria. Despite a wide range of solid-state materials, including 2D materials, there is still a need for high performance H2 storage. To address this issue, volumetric experimental set-up will be used for industrial test benches and characterize hydrogen storage. Ab initio calculations coupled to molecular dynamics (AIMD) will support experimental measurements from modelization of the adsorption sites to explain isotherm experiments. Then, a technical-economic study will be conducted to position aminated h-BN nanosheets for H2 storage.
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Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. 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Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. Provider Academic Bibliometrics & Assessment Computational Utility Service Expiration Session Name greekSession Description Stores the user session ID for Academic Bibliometrics & Assessment Computational Utility Service. 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